○ 著　書（Books）

(1) ブレンドの相構造のキャラクタリゼーション
　　入門　高分子特性解析、６章
共立出版 1984.6.10, pp.216-234.
（橋本竹治、柴山充弘、河合弘廸）

(2) ブロックおよびグラフト共重合体のミクロ相分離機構、相分離構造とその応用
新しい複合材料と先端技術、第２部　４．３節
　東京化学同人, 1986.12.15, pp.103-113.
（柴山充弘、橋本竹治）

(3) Microdomain Separation and the Polymer-Polymer Interface in Block Copolymers.
in "Block Copolymers: Science and Technology", D.J. Meier Ed.
pp. 63-108, MMI Press, Harwood Academic Publishers, 1983.
(T.Hashimoto, M.Shibayama, M.Fujimura, H.Kawai)

(4) Characterization of Gel Structure by Means of SAXS and SANS.
in "Polymer Gels", D. Rossi, K. Kajiwara, Y. Osada, and A. Yamauchi Eds.
pp. 3-11, Plenum, N.Y., 1991.
(K. Kajiwara, S. Kohjiya, M. Shibayama, H. Urakawa)

(5) 高分子機能材料、第３巻高分子物性の基礎、２．２．１Ｃ節、
　　共立出版、pp.121-128、1993.　
（柴山充弘）

(6) Volume Phase Transition and Related Phenomena of Polymer Gels
　　in "Responsive Gels: Volume Transitions I",
　　Adv. Polym. Sci., vol.109, 1-62. Springer-Verlag, 1993.
(M. Shibayama, T. Tanaka)

(7) Poly(vinyl alcohol)-Ion Complex Gels, "The Polymeric Materials Encyclopedia:
Synthesis Properties and Applications", vol. 9, 1996, 7020-7026, CRC Press, FL.
(M. Shibayama)

(8) 大学院高分子科学、＜構造編＞、3.5節
　　多成分系の凝集構造、講談社, pp. 103 - 136, 1997.
　（柴山充弘）

(9) ゲルハンドブック　第１編　基礎編、第２章３節２．
　　膨潤の速度論、エヌ・ティー・エス出版、pp.48-55, 1997.
（柴山充弘）

(10) Multi-Phases in Polymeric Gels in "Structure and Properties of Multi-Phase
　　Polymeric Materials",
T. Araki, Q. Tran-Cong, and M. Shibayama Eds., Marcel Dekker, 1998,
Chapt. 6, pp. 195 -231
(M. Shibayama)

(11) In-situ Studies on Gelation by Dynamic and Time-Resolved Light Scattering
Technique
in "The Wiley Polymer Networks Group Review", Vol. 2, pp. 3-13.
B. T. Stokke and A. Elgsaeter Eds., Wiley, 1999.
(M. Shibayama, T. Norisuye, M. Takeda)

(12) Anomalous Cross-Link Density Dependence of Spatial Inhomogeneities in
Polymer Gels
in "The Wiley Polymer Networks Group Review", Vol. 2, pp. 383-392.
B. T. Stokke and A. Elgsaeter Eds., Wiley, 1999.
(F. Ikkai, M. Shibayama)

(13) Neutron Scattering in "Experimental Methods in Polymer Science", Chapt. 2,
pp. 57-154.
T. Tanaka Ed., Academic Press, NY, 2000.
(M. Shibayama, H. Jinnai, T. Hashimoto)

(14) Real-Time Observation of Gelation and Vitrification in "Statistical Physics",
M. Tokuyama and H. E. Stanley Eds. American Institute of Physics,
pp. 158-163 , 2000
(M. Shibayama, S. Ozeki, and T. Norisuye)

(15) Kinetic theory of Swelling
in "Gel Handbook" Academic Press, NY, 2000, in press.
(M. Shibayama)

(16) 有機無機複合体のキャラクタリゼーションの新しい取り組み
　　高分子科学と無機化学とのキャッチボール
　　エヌ・ティー・エス出版、2001
（柴山充弘）

○学術論文 (Original Papers) 　 　　
(1) Microdomain Size of Styrene-Isoprene Block Copolymers and Unperturbed Chain
Dimension of Polyisoprene Having 1,2- and 3,4-Linkages.
Macromol. Sci. Phys., vol.B17, 1980.9, pp.389-406.
(T.Hashimoto, N.Nakamura, M.Shibayama, A.Izumi, H. Kawai)

(2) Domain-Boundary Structure of Styrene-Isoprene Block Copolymer Films Cast from Solution. 4. Molecular Weight Dependence of Lamellar Microdomains.
Macromolecules, vol.13, 1980.9, pp.1237-1247.
(T.Hashimoto, M.Shibayama, H.Kawai)

(3) An Apparatus for High Speed Measurements of Small-Angle X-ray Scattering
Profiles with a Linear Position Sensitive Detector.
Polym. J., vol.13, 1981.9, pp.501-516.
(T.Hashimoto, S.Suehiro, M.Shibayama, K.Saijo, H.Kawai)
　　　　　　　　　　　　　　　　
(4) Microdomain Strucuture of an ABC-Type Triblock Polymer of Polystyrene-
Poly[(4-vinylbenzyl)dimethylamine)]-Polyisoprene Cast from Solution.
Macromolecules, vol.15, 1982.3, pp.274-280.
(M.Shibayama, H.Hasegawa, T.Hashimoto, H.Kawai)

(5) Rheological and Morphological Behavior of Styrene-Butadiene Diblock Solutions in Selective Solvents.
J. Rheology, vol.26, 1982.3, pp.153-179.
(H.Watanabe, T.Kotaka, T.Hashimoto, M.Shibayama, H. Kawai)

(6) Ordered Structure in Block Polymer Solutions. 1. Selective Solvents.
Macromolecules, vol.16, 1983.1, pp.16-28.
(M.Shibayama, T. Hashimoto, H.Kawai)

(7) Ordered Structure in Block Polymer Solutions. 2. Its Effect on Rheological
Behavior.
Macromolecules, vol.16, 1983.3, pp.361-371.
(T. Hashimoto, M.Shibayama, H.Kawai, H.Watanabe, T.Kotaka)

(8) Ordered Structure in Block Polymer Solutions. 4. Scaling Rules on Size of
Fluctuations with Block Molecular Weight, Concentration, and Temperature in Segregation and Homogeneous Regimes.
Macromolecules, vol.16, 1983.7, pp.1093-1101.
(T.Hashimoto, M.Shibayama, H.Kawai)

(9) Ordered Structure in Block Polymer Solutions. 3. Concentration Dependence of
Microdomains in Non-Selective Solvents.
Macromolecules, vol.16, 1983.9, pp.1427-1433.
(M.Shibayama, T.Hashimoto, H.Hasegawa, H.Kawai)

(10) Ordered Structure in Block Polymer Solutions. 5. Equilibrium and Non-
Equilibrium Aspects of Microdomain Formation.
Macromolecules, vol.16, 1983.9, pp.1434-1443.
(M.Shibayama, T.Hashimoto, H.Kawai)

(11) Neutron Cloud Points and Concentration Fluctuations of Polymer Blends.
Polym. Bull., vol.12, 1984, pp.7-12.
(H. Yang, M. Shibayama, R.S. Stein, C.C. Han)

(12) Confined-Chain Statistics of Block Polymers and Estimation of Optical
Anisotropy and Domain Size.
Macromolecules, vol.18, 1985.10, pp.1855-1864.
(T.Hashimoto, M.Shibayama, H.Kawai, D.J.Meier)

(13) Study of Miscibility and Critical Phenomena of Deuterated Polystyrene and
Hydrogenated Poly(vinyl methyl ether) by Small Angle Neutron Scattering.
Macromolecules, vol.18, 1985.11, pp.2179-2187.
(M.Shibayama, H.Yang, R.S.Stein, C.C.Han)

(14) Small-Angle X-ray Scattering Analyses of Lamellar Microdomains Based on a
Model of One-Dimensional Paracrystal with Uniaxial Orientation.
Macromolecules, vol.19, 1986.3, pp.740-749.
(M.Shibayama, T.Hashimoto)

(15) Time-Resolved SAXS Studies on Kinetics of Order-Disorder Transition of Block
Polymers. 1. Experimental Technique.
Macromolecules, vol.19, 1986.3, pp.750-754.
(T.Hashimoto, K.Kowsaka, M.Shibayama, H.Kawai)

(16) Time-Resolved SAXS Studies on Kinetics of Order-Disorder Transition of Block
Polymers. 2. Temperature and Concentration Dependence.
Macromolecules, vol.19, 1986.3, pp.754-762.
(T.Hashimoto, K.Kowsaka, M.Shibayama, H.Kawai)

(17) Deuteration Effects on the Miscibility and Phase Separation Kinetics of Polymer Blends.
Macromolecules, vol.19, 1986.6, pp.1667-1674.
(H.Yang, M.Shibayama, R.S.Stein, N.Shimizu, T.Hashimoto)

(18) Structure and Properties of Fatigued Segmented Poly(urethaneureas).
I. Segment Orientation Mechanism due to Fatigue.
Polym. J., vol.18, 1986.10, pp.719-733.
(M.Shibayama, T.Kawauchi, T.Kotani, S.Nomura)

(19) Structure and Properties of Fatigued Segmented Poly(urethaneurea)s.
II. Structural Analyses of Fatigue Mechanism.
Polym. J., vol.19, 1987.9, pp.1067-1080.
(M.Shibayama, Y.Ohki, T.Kotani, S. Nomura)

(20) 11B NMR Study on the Reaction of Poly(vinyl alcohol) with Boric Acid.
Polymer(London), vol.29, 1988.2, pp. 336-340.
(M.Shibayama, M.Sato, Y.Kimura, H.Fujiwara, S.Nomura)

(21) Sol-Gel Transition of Poly(vinyl alcohol)-Borate Complex
Polymer(London), vol.29, 1988.11, pp.2066-2071.
(M. Shibayama, H. Yoshizawa, H. Kurokawa, H. Fujiwara, S. Nomura)

(22) Preparation of High Strength Poly(vinyl alcohol) Fibers by Crosslinking Wet
Spinning.
J. Appl. Poly. Sci., vol.37, 1989, pp.1403-1414.
(H. Fujiwara, M. Shibayama, J.H. Chen, S. Nomura)

(23) Structure and Properties of Fatigued Segmented Poly(urethaneurea)s
III. Quantitative Analyses of Hydrogen Bond.
Polym. J., vol.21, 1989.11, pp.895-903.
(T. Yamamoto, M. Shibayama, S. Nomura)

(24) Asymptotic Behavior and Lorentz Factor for Small-Angle Elastic Scattering
Profiles from Preferentially Oriented Asymmetric Bodies.
J. Appl. Phys., vol.66, 1989.11, 4188-4197.
(M. Shibayama, S. Nomura, T. Hashimoto, E.L. Thomas)

(25) 架橋型湿式紡糸法による高強力ポリビニルアルコール繊維の構造と物性　
Ｉ．力学的および熱的性質
繊維学会誌、vol.46, 1990.1, pp.15-20.
(柴山充弘、早崎忠義、陳景輝、野村春治、藤原弘史)
Structure and Properties of High Strength Poly(vinyl Alcohol) Fibers Prepared by
Cross-linking/Wet Spinning. I. Mechanical and Thermal Properties.
Sen-i Gakkaishi, vol.46, 1990.1, pp.15-20.
(M. Shibayama, T. Hayasaki, J.H. Chen, S. Nomura, H. Fujiwara)

(26) Structure and Orientational Behaviour of Polyurethane Containing
Polydimethylsiloxane.
Polymer, vol.31, 1990.4, 749-757.
(M. Shibayama, M. Inoue, T. Yamamoto, S. Nomura)

(27) Small-Angle Neutron Scattering Studies on Chain Asymmetry on Coextruded
Poly(vinyl alcohol) Films.
Macromolecules, vol.23, 1990.5, 1438-1443.
(M. Shibayama, H. Kurokawa, S. Nomura, S.K. Roy, R.S. Stein, W. Wu)

(28) Physical Gels of Aqueous Poly(vinyl alcohol) Solutions: A Small-Angle
Neutron-Scattering Study.
Macromolecules, vol.23, 1990.8, 2245-2251.
(W. Wu, M. Shibayama, S. Roy, H. Kurokawa, L.D. Coyne, S. Nomura,
R.S. Stein)

(29) 架橋型湿式紡糸法による高強力ポリビニルアルコール繊維の構造と分子
配向評価
繊維学会誌、vol.47, 1991.1, 5-10.
(早崎忠義、柴山充弘、桜井伸一、野村春治、藤原弘史、末広祥二)
Structure and Molecular Orientation of High Strength Poly(vinyl alcohol) Fibers
Prepared by Crosslinking/Wet Spinning.
Sen-i Gakkaishi, vol.47, 1991.1, 5-10.
(T. Hayasaki, M. Shibayama, S. Sakurai, S. Nomura, H. Fujiwara)

(30) Transparency of Recycled Polypropylene film.
J. Appl. Polym. Sci., vol.42, 1991.5, 1451-1458.
(M. Shibayama, K. Imamura, K. Katoh, S. Nomura)

(31) Bulk and Surface Characterization of Cellulose/Poly(vinyl alcohol) blends by
FTIR.
Polymer, vol.32, 1991.6, 1010-1016.
(M. Shibayama, T. Yamamoto, C. Xiao, S. Sakurai, A. Hayami, S. Nomura)

(32) Structure of High Transparent Polypropylene Film.
Polym. J., vol.23, 1991.7, 837-846.
(M. Shibayama, K. Katoh, T. Iwamoto, D. Takahashi, S. Nomura)

(33) Structure and Properties of Fatigued Segmented Poly(urethaneurea)s
IV. Dynamic Infrared Dichroism.
Polym. J., vol.23, 1991.4, 311-320.
(T. Yamamoto, M. Shibayama, S. Nomura)

(34) Structure Characterization of Polyurethanes Containing Poly(dimethyl Siloxane).
Macromolecules, vol.24, 1991.23, 6254-6262.
(M. Shibayama, M. Suetsugu, S. Sakurai, T. Yamamoto, S. Nomura)

(35) Infrared Dichroism Study of Segmented Polyurethaneurea with Triblock Polyether Soft Segments.
Polym. J., vol.23, 1991.8, 991-998.
(S. Kohjiya, Y. Ikeda, S. Yamashita, M. Shibayama, T. Kotani, S. Nomura)

(36) ホウ酸架橋によるポリビニルアルコールゲルフィルムの構造と物性
　　繊維学会誌、vol. 48, 1992.2, 74-83.
（佐野真弘、柴山充弘、桜井伸一、黒川秀信、野村春治）
Sen-i Gakkaishi, vol. 48, 1992.2, 74-83.
　　Structure and Properties of Borate Crosslinked Poly(vinyl alcohol) Gel films.
(M. Sano, M. Shibayama, S. Sakurai, H. Kurokawa, S. Nomura)

(37) Effects of Critical Concentration Fluctuations on the Photocyclization of a
bichromophoric Molecule in the One-Phase Region of Polystyrene/Poly(vinyl
methyl ether) Blends.
(Q. Tran-Cong, K. Meisyo, O. Yano, T. Soen, M. Shibayama)
Macromolecules, vol. 23, 1992.9, 2330-2335.

(38) Phase behaviour and Sol-Gel Transition of Poly(vinyl alcohol)-Borate Complex.
Polymer, vol. 33, 1992.10, 2182-2187.
(H. Kurokawa, M. Shibayama, T. Ishimaru, W. Wu, S. Nomura)

(39) Small-Angle Neutron Scattering from Poly(vinyl alcohol)-Borate Gels.
Polymer, vol. 33, 1992.14, 2883-2890.
(M. Shibayama, M. Muthukumar, H. Kurokawa, S. Roy, S. Nomura, R.S. Stein)

(40) Super-Absorbency and Phase Transition of Gels in Physiological Salt Solutions.
Nature, vol.160, 1992.1660, 142-144.
(Y.-Z. Zhang, T. Tanaka, M. Shibayama)

(41) Small Angle Neutron Scattering Study on Poly(N-isopropyl acrylamide) gels Near Their Volume-Phase Transition Temperature.
J. Chem. Phys., vol.97, 1992,9, 6829-6841.
(M. Shibayama, T. Tanaka, C.C. Han)

(42) Small-Angle Neutron Scattering Study on Weakly Charged Temperature Sensitive Polymer Gels.
J. Chem. Phys., vol.97, 1992,9, 6842-6854.
(M. Shibayama, T. Tanaka, C.C. Han)

(43) 末端架橋型ポリテトラヒドロフランネットワークの構造と物性
　　 高分子論文集、vol.49, 1992.11, 907-914.
　 （高橋啓司、桜井伸一、中山美矢、乾洋治、柴山充弘、橋本保、野村春治）
Structure and Properties of End-Crosslinked Poly(tetrahydrofuran) Network.
Kobunshi Ronbunshu, vol.49, 1992.11, 907-914.
(K. Takahashi, S. Sakurai, M. Nakayama, Y. Inui, M. Shibayama, T. Hashimoto,
S. Nomura)

(44) Morphology Transition from Cylindrical to Lamellar Microdomains of Block
Copolymers.
Macromolecules, vol.23, 1993.3, 485-491.
(S. Sakurai, T. Momii, K. Taie, M. Shibayama, S. Nomura, T. Hashimoto)

(45) Gelation of Poly(vinyl alcohol)-Vanadate Aqueous Solutions.
Macromolecules, vol.26, 1993.4, 623-627.
(M. Shibayama, M. Adachi, F. Ikkai, H. Kurokawa, S. Sakurai, S. Nomura)

(46) Effects of Microdomain Structures on Molecular Orientation of
Poly(styrene-block-butadiene-block-styrene) Triblock Copolymers.
Macromolecules, vol.26, 1993.13, 3351-3356.
(S. Sakurai, J. Sakamoto, M. Shibayama, S. Nomura)

(47) Controlling Morphology of PS/PVME Blends Undergoing Spinodal
Decomposition Process by Photo-Cross-Links.
Polym. Eng. Sci., vo.33, 1993.12, 772-780.
(Q. Tran-Cong, M. Imura, O. Yano, T. Soen, M. Shibayama)

(48) ランダム位相近似によるスチレン系熱可塑性エラストマーの成膜実験結果
の解釈
　　 日本ゴム協会誌、 vol.66, 1993.7, 483-487.
Analysis of the Experimental Results of the Effect of Solvent Evaporation Rate by Random Phase Approximation.
J. Soc. Rubber Ind. Jpn., vol.66, 1993.7, 483-487.
(S. Kohjiya, T. Yamato, Y. Miyake, M. Shibayama)

(49) ESCAによるセルロース／ポリビニルアルコールブレンドフィルムのデプ
スプロファイリング
繊維学会誌、vol.49, 1993.9 466-473.
（奥村治樹、柴山充弘、越崎寛之、櫻井伸一、野村春治）
　　ESCA Study on Depth Profiling of Cellulose/Poly(vinyl alcohol) Blend Films.
Sen-i Gakkaishi, vol.49, 1993.9 466-473.
(H. Okumura, M. Shibayama, H. Koshizaki, S. Sakurai, S. Nomura)

(50) Small-angle Neutron Scattering Study on Poly(N-isopropyl acrylamide-co-acrlyic acid) Copolymer Solutions.
J. Physique (Paris) IV, Colloque C8, vol.3, 1993, 25-28.
(M. Shibayama, T. Tanaka, C.C. Han)

(51) Peeling of Laminated Films Comprising High-Density Polyethylene and
Polypropylene/Low-Density Polyethyene blends.
Polymer, vol. 35, 1994.2, 271-280.
(M. Shibayama, A. Izutani, A. Ishikawa, K. Tanaka, S. Nomura)

(52) Changes in Structure and Properties Due to Mechanical Fatigue for Polyurethanes Containing Poly(dimethyl siloxane).
Polymer, vol.35, 1994.3, 532-539.
(S. Sakurai, S. Nokuwa, M. Morimoto, M. Shibayama, S. Nomura)

(53) Complexation of Poly(vinyl alcohol)-Congo Red Aqueous Solutions. I. Viscosity
Behavior and Gelation Mechanism
Macromolecules, vol.27, 1994.7, 1738-1743.
(M. Shibayama, F. Ikkai, R. Moriwaki, S. Nomura)

(54) Isothermal Crystallization of End-linked Poly(tetrahydrofuran) Networks.
Polymer, vol.35, 1994.14, 2944-2951.
(M. Shibayama, H. Takahashi, H. Yamaguchi, S. Sakurai, S. Nomura)

(55) Phase Separation Induced Mechanical Transition of Poly(N-isopropylacrylamide)/Water Isochore Gels.
Macromolecules, vol. 27, 1994.18,5060-5066.
(M. Shibayama, M. Morimoto, S. Nomura)

(56) Swelling/Shrinking and Dynamic Light Scattering Studies on Chemically
Cross-linked Poly(vinyl alcohol) Gels in the Presence of Borate Ions.
Macromolecules, vol. 27, 1994.19,5350-5358.
(M. Shibayama, T. Takeuchi, S. Nomura)

(57) Complexation of Poly(vinyl alcohol)-Congo Red Aqueous Solutions.
II. SANS and SAXS Studies on Sol-Gel Transition.
Macromolecules, vol. 27, 1994.22,6383-6388.
( M. Shibayama, F. Ikkai, S. Nomura)

(58) Viscosity Behavior of Weakly Charged Polymer Ion Complexes Comprising
Poly(vinyl alcohol) and Congo Red.
Polymer, vol.35, 1994.26, 5716-5721.
(M. Shibayama, R. Moriwaki, F. Ikkai, S. Nomura )

(59) エチレンビニルアルコールランダムコポリマーのほう酸架橋型フィルムの
　　構造と物性
　　繊維学会誌、 vol.51, 1995.1 43-50.
（高岸正也、柴山充弘、野村春治）
　　Strucuture and Properties of Poly(ethylene-ran-vinyl alcohol) Films Crosslinked With Borate Ions.
Sen-i Gakkaishi, vol.51, 1995.1, 43-50.
(M. Takagishi, M. Shibayama, S. Nomura)

(60) Microscopic Structure and Viscosity Behaviors of Ion-complexed Polymer Gels.
Macromol. Symp., vol. 93, 1995 277-281.
(M. Shibayama, F. Ikkai, S. Nomura )

(61) Small-angle Neutron Scattering Study on Weakly Charged Poly(N-isopropyl
acrylamide-co-acrylic acid) Copolymer Solutions
J. Chem. Phys., vol.102, 1995.23, 9392-9400.
(M. Shibayama, T. Tanaka)

(62) Isothermal Crystallization of End-linked Poly(tetrahydrofuran) Networks
II. Molecular Weight Dependence
Macromolecules, vol. 28, 1995.16,5547-5553.
( H. Takahashi, M. Shibayama, M. Hashimoto, S. Nomura)

(63) 有機溶媒を用いた再生セルロース繊維の紡糸とその特性解析
Regenerated Cellulose Fibers Spun from Organic Solvent
Sen-i Gakkaishi, vol.51, 1995.9, 422-431.
(S. Cho, M. Kamata, A. Hayami, M. Shibayama, S. Nomura)

(64) Small-Angle Neutron Scattering Study on End-linked Poly(tetrahydrofuran)
Networks.
Macromolecules, vol. 28, 1995.20,6860-6864.
(M. Shibayama, H. Takahashi, S. Nomura)

(65) Miscibility and Crystallinity Control of Nylon 6 and Poly(m-xylene adipamide)
Blends
Polymer, vol. 36, 1995.25,4811-4816.
(M. Shibayama, K. Uenoyama, J. Oura, T. Iwamoto, S. Nomura )

(66) Equilibrium Swelling and Small-angle Neutron Scattering Studies on End-linked
Poly(tetrahydrofuran) Networks.
Macromolecules, vol. 28, 1995.26,8824-8828.
(H. Takahashi, M. Shibayama, H. Fujisawa, S. Nomura)

(67) Analogy between Swelling and Viscosity Behavior of Ion-Complexed Poly(vinyl
alcohol) in Aqueous Media.
Macromolecules, vol. 29, 1996.3, 885-891.
(M. Shibayama, M. Uesaka, S. Inamoto, S. Nomura)

(68) Complexation of Poly(vinyl alcohol)-Congo Red Aqueous Solutions. 3. Dynamic
Light Scattering Studies on Sol-Gel Transition.
J. Polym. Sci., Polym. Phys. Ed., vol. 34, 1996.5, 939-945.
( F. Ikkai, M. Shibayama, S. Nomura, and C.C. Han)

(69) Thermal Properties of Copolymer Gels Containing N-isopropylacrylamide
Macromolecules, vol. 29, 1996.6, 2019-2024.
(M. Shibayama, S. Mizutani, S. Nomura)

(70) Microscopic Inhomogeneities in Weakly-charged Temperature Sensitive Polymer Gels and Solutions.
Macromol. Symp., vol. 106, 1996 (April), 337-343.
(M. Shibayama)

(71) ナイロン６/芳香族ポリアミドブレンドフィルムの力学物性と構造
Mechanical Properties and Structure of Nylon6/Aromatic Polyamide Blend Film
高分子論文集、vol. 53, 1996.7, 455-462.
（大浦純一、柴山充弘、櫻井伸一、野村春治、岩本壮弘）

(72) Microstructure and Swelling Behavior of Ion-Exchange Resin.
J. Polym. Sci., Polym. Phys. Ed., vol. 34, 1996.9, 1637-1645.
(F. Ikkai, M. Shibayama)

(73) Swelling/Shrinking Kinetics of Chemically Cross-linked Poly(vinyl alocohol) Gels in the Presence of Borate Ions.
J. Chem. Phys., vol. 105, 1996.10, 4350-4357.
(M. Shibayama, M. Uesaka, Y. Shiwa)

(74) pH and Salt Concentration Dependence of the Microstructure of Poly(N-
isopropylacrylamide-co-acrylic acid) Gels.
J. Chem. Phys., vol. 105, 1996.10, 4358-4366.
(M. Shibayama, F. Ikkai, S. Inamoto, S. Nomura, C. C. Han)

(75) Dynamic Light Scattering Study on Poly( N-isopropylacrylamide-co-acrlyic acid) Gels.
Macromolecules, vol. 29, 1996.20, 6535-6540.
(M. Shibayama, Y. Fujikawa, S. Nomura)

(76) Structure Relaxation of Hydrophobically Aggregated Poly(N-isopropyl acrylamide) in Water
Macromolecules, vol. 29, 1996.21, 6966-6968.
(M. Shibayama, Y. Suetoh, S. Nomura)

(77) ポリマーネットワークの結晶化における架橋密度および結晶化温度依存性
Crosslinking Density and Temperature Dependence of Crystallization Kinetics of
Polymer Networks.
高分子論文集、vol. 53, 1996.11, 722-728.
（橋本　学、柴山充弘、高橋啓司、野村春治）

(78) Cross-link Density Dependence of Spatial Inhomogeneities and Dynamic
Fluctuations of Poly(N-isopropylacrylamide) Gels
Macromolecules, vol. 29, 1996.27, 8746-8750.
(M. Shibayama, T. Norisuye, S. Nomura).

(79) SAXS and Dynamic Viscoelastic Studies on Segmented Polyurethaneurea
Solutions.
Polymer, vol. 38, 1997.4, 769-774.
(F. Ikkai, M. Shibayama, H. Kashiwara, S. Nomura)

(80) Anomalous cross-link density dependence of scattering from charged gels
Phys. Rev. E, Rapid Commun., vol. 56, 1997.1, R51-R54.
(F. Ikkai, M. Shibayama)

(81) Ｎ-イソプロピルアクリルアミドゲルの脱疎水水和の熱解析
- 調製温度依存性 -
Thermal Analysis of N-isopropylacrylamide Gels.
Preparation Temperature Dependence
繊維学会誌、vol. 53, 1997.8, 455-462.
(柴山　充弘、中川　智太、末藤　陽介、野村　春治)
　 Sen-i Gakkai Shi, vol. 53, 1997.8, 455-462.
(M. Shibayama, T. Nakagawa, Y. Suetoh, and S. Nomura)

(82) Effect of Degree of Cross-linking on Spatial Inhomogeneity in Charged Gels.
I. Theoretical Prediction and Light Scattering Study
J. Chem. Phys., vol.107, 1997.13, 5227-5235.
(M. Shibayama, F. Ikkai, Y. Shiwa, Y. Rabin)

(83) Simple Scaling Rules on Swollen and Shrunken Gels
Macromolecules, vol.30, 1997.23, 7307-7312.
(M. Shibayama, Y. Shirotani, H. Hirose, and S. Nomura)

(84) Static Inhomogeneities and Dynamic Fluctuations of Temperature Sensitive
Polymer Gels.
Physica A, vol.249, 1998, 245-252.
(M. Shibayama, S. Takata, and T. Norisuye)

(85) Comparison of the Experimental and Theoretical Structure Factors of Temperature Sensitive Polymer Gels
Macromolecules, vol.31, 1998.5, 1608-1614.
(M. Shibayama, K. Kawakubo, T. Norisuye)

(86) Small-angle Neutron Scattering Study on Charged Gels in Deformed State.
Macromolecules, vol.31, 1998.8, 2586-2592.
(M. Shibayama, K. Kawakubo, F. Ikkai, and M. Imai)

(87) Time Resolved Light Scattering Study on the Gelation Process of Poly(N-isopropyl acrylamide).
Polymer, vol.39, 1998.8, 2769-2775.
(T. Norisuye, M. Shibayama, S. Nomura)

(88) Effect of Degree of Cross-linking on Spatial Inhomogeneity in Charged Gels.
2. Small-angle Neutron Scattering Study.
Macromolecules, vol.31, 1998.10, 3275-3281.
(F. Ikkai, M. Shibayama, and C. C. Han)

(89) Isothermal crystallization of end-linked poly(tetrahydrofuran) networks. 3. Small-angle neutron scattering.
Polymer, vol.39.16, 3759-3776 (1998).
(M. Shibayama, H. Takahashi, S. Nomura, M. Imai)

(90) Cluster-size Distribution of Cross-linked Polymer Chains Across the Gelation
Threshold Macromolecules, vol.31, 1998.16, 5316-5322.
(T. Norisuye, M. Takeda, M. Shibayama)

(91) Kinetics of Volume Phase Transition in Poly(N-isopropylacrylamide-co-acrylic acid) Gels
Macromolecules, vol.31, 1998.16, 5336-5342.
(H. Hirose and M. Shibayama)

(92) 高分子物理ゲルの微視的構造不均一性
　　高分子論文集、vol. 55, 1998.10, 633-636.
(F. Ikkai, M. Shibayama)

(93) Effect of Degree of Cross-linking on Spatial Inhomogeneity in Charged Gels.
3. Ionization Effect.
Macromolecules, vol.31, 1998.24, 8526-8530.
(F. Ikkai, O. Iritani, and M. Shibayama)

(94) Time Resolved Dynamic Light Scattering Studies on Gelation Process of Organic-Inorganic Polymer Hybrid
Macromolecules, vol.32, 1999.5, 1528-1533.
(T. Norisuye, M. Shibayama, R. Tamaki, and Y. Chujo)

(95) Effects of electrokinetic-chromatography conditions on the structure and properties of polyallylamine-supported pseudo-stationary phase: A study by dynamic light scattering.
J. Chromatography A, vol.836, 1999, 295-303.
(N. Tanaka, K. Nakagawa, H. Nagayama, K. Hosoya, T. Ikegami, A. Itaya, and M.
Shibayama)

(96) Anisotropic Scattering Profiles of Charged Gels in Deformed State
Phys. Rev. E., vol.59, 1999.5, 5891-5894.
(Y. Shiwa, M. Shibayama)

(97) Static Inhomogeneities in Thermoreversible Physical Gels
Phys. Rev. Lett., vol.82, 1999.24, 4946-4949.
(F. Ikkai, M. Shibayama)

(98) Preparation Temperature Dependence and Effects of Hydrolysis on
Static Inhomogeneities of Poly(acrylamide) Gels.
Macromolecules, vol.32, 1999.12, 3989-3993.
(Shin-ichi Takata, Tomohisa Norisuye,M. Shibayama)

(99) Dynamics of Probe Particles Trapped in Polymer Solutions and in Polymer Gels
Macromolecules, vol.32, 1999.21, 7086-7092.
(M. Shibayama, Y. Isaka, Y. Shiwa)

(100) Shrinking Kinetics of Poly(N-isopropylacrylamide) Gels T-jumped Across Its
Volume Phase Transition Temperature
Macromolecules, vol.32, 1999.22, 7461-7468.
(M. Shibayama, K. Nagai)

(101) Effects of Non-uniform Solvation on Thermal Response in Poly(N-
isopropylacrylamide) Gels
Polymer, vol.41, 2000.2, 505-510.
(Y. Suetoh, M. Shibayama)

(102) Static Inhomogeneities and Dynamics of Swollen and Reactor-Batch Polymer
Gels
J. Chem. Phys., vol.112, 2000.1, 442-449.
(M. Shibayama, Y. Shirotani, Y. Shiwa)

(103) Time-Resolved Dynamic Light Scattering Study on the Dynamics of Silica Gels during Gelation Process.
Macromolecules, vol.33, 2000.3, 900-905.
(T. Norisuye, M. Inoue, M. Shibayama, R. Tamaki, Y. Chujo)

(104) Critical Dynamics of Cross-linked Polymer Chains near Gelation Threshold
Macromolecules., vol.33, 2000.8, 2909-2915.
(M. Takeda, T. Norisuye, M. Shibayama)

(105) Heat-Induced Gelation of b-Lactoglobulin. 1. Time-Resolved Dynamic Light
Scattering.
Macromolecules, vol.33, 2000.15, 5470-5475.
(S. Takata, T. Norisuye, N. Tanaka, M. Shibayama)

(106) Static Inhomogeneities in Physical Gels: Comparison of Temperature-induced and Concentration-induced Sol-Gel Transition
Macromolecules, vol.33, 2000.21, 7868-7876.
(M. Shibayama, M. Tsujimoto, F. Ikkai)

(107) Preparation Pressure Dependence of Structure Inhomogeneities and Dynamic
Fluctuations in Poly(N-isopropylacrylamide) Gels
(C. Nakamoto, T. Motonaga, M. Shibayama)
Macromolecules, vol.34, 2001.4, 911-917.

(108) Characterization of Gel Structure in Poly(vinyl chloride) by Light Scattering
1. Molecular Weight and Process Temperature Dependence.
Polymer, vol.42, 2001.8, 3875-3881.
(T. Kawauchi, M.Isshiki, M. Takeda, M. Shibayama)

(109) Multiple Phase Behavior and Its Microscopic Implication of 4-
Acrylamidosalicylic Acid Gel
J. Chem. Phys, vol.114, 2001.15, 6906-6912.
(M. Annaka, M. Shibayama, F. Ikkai, M. Sugiyama, T. Nakahira, T. Tanaka)

(110) Formation of ordered macropores and templated nanopores in silica sol-gel
system incorporated with EO-PO-EO triblock copolymer
Colloids and Surfaces A: Physicochem. And Eng. Aspects, vol. 187-188, 117-122
(2001)
(Yosuke Sato, Kazuki, Nakanishi, Kazuyuki Hirao, Hiroshi Jinnai, Mitsuhiro
Shibayama, Yuri B. Melnichenko, George D. Wignall)

(111) SANS Studies on Frozen Inhomogeneities and Local Structure in Polymer Gels
J. Phys. Soc. Jpn., vol.70, Suppl. A, 306-310 (2001).
(M. Shibayama, T. Norisuye, F. Ikkai)

(112) Studies on pH and Temperature Dependence of the Dynamics and Heterogeneities
in Poly(N-isopropyl acrylamide-co-Sodium Acrylate) Gels
Polymer, vol. 42, 8925-8934 (2001).
(T. Motonaga, M. Shibayama)

(113) Dynamic Light Scattering Study on Gelatin Aqueous Solutions and Gels
J. Chem. Phys. Vol. 115, 2001.9, 4285 - 4291.
(M. Shibayama, M. Okamoto)

(114) Time-Resolved Dynamic Light Scattering Study on Gelation and Gel-Melting
Processes of Gelatin Gels
Macromolecules, Vol. 34, 2001.24, 8496 - 8502.
(M. Okamoto, T. Norisuye, M. Shibayama)

(115) Dynamic Light Scattering Study on Reentrant Sol-Gel Transition of Poly(vinyl
alcohol)-Congo Red Complex in Aqueous Media
Macromolecules, in press.
(M. Tsujimoto, M. Shibayama)

(117) Dependence of Shrinking Kinetics of Poly(N-isopropylacrylamide) Gels on
Preparation Temperature
Polymer, in press.
(S. Takata, T. Norisuye, M. Shibayama)

(118) Small-angle Neutron Scattering Study on Selective Solvation of Poly(12-acryloyloxydocecanoic acid-co-acrylic acid) in Mixed Solvents
Langmuir, submitted.
(N. Masui, F. Ikkai, T. Karino, S. Naito, S. Kunugi, K. Kurita, M. Shibayama)

(119) Small-angle Neutron Scattering Study on Preparation Temperature Dependence of
Thermosensitive Gels
(S. Takata, T. Norisuye, M. Shibayama)
Macromolecules, submitted.

(120) Small Angle Neutron Scattering Studies on Structural Inhomogeneities of
Randomm Cross-linked Polymer Gels: Comparison with Chemically Cross-linked
Gels.
Polymer, submitted.
(T. Norisuye, N. Masui, M. Shibayama, S. Panyukov)

(121) Real-Time Dynamic Light Scattering on Gelation and Vitrification
Macromolecules, to be submitted.
(M. Shibayama, S. Ozeki, T. Norisuye)

(122) Structure Characterization of Hairy Nanoparticles Consisting of Hydrophobic Core and Thermosensitive Hairs
Macromolecules, submitted.
(S. Takata, M. Shibayama, R. Sasabe, H. Kawaguchi)

(123) Heat-induced Self-assembling of Thermosensitive Block Copolymer
I. Small-angle Neutron Scattering Study
Macromolecules, submitted.
(S. Okabe, M. Shibayama, S. Sugihara, S. Aoshima)

○参考報文（Review Papers）　
(1) Microdomain Separation of Block Polymers.
Mem. Fac. Engr. Kyoto Univ., vol.43(2), 1981, pp.184-223.
(T.Hashimoto, M.Shibayama, M.Fujimura, H.Kawai)
　
(2) ブレンドの相構造のキャラクタリゼーション 　
高分子, vol.31, 1982.9, pp.871-877.
　（橋本竹治、柴山充弘、河合弘廸） 　

(3) Structural Changes in Fatigued Segmented Poly(urethaneureas).
Repts. Progr. Polym. Phys. Jpn., vol.29, 1986, pp.289-292.
(T. Kawauchi, T. Kotani, M. Shibayama, S. Nomura)

(4) 同位体高分子間の相分離
　 化学と工業、vol.40, 1987.9, pp.791-793.
（柴山充弘）

(5) Dynamic Infrared Dichroism of Segmented Poly(urethaneurea).
Repts. Progr. Polym. Phys. Jpn., vol.30, 1987, pp.541-544.
(T. Yamamoto, M. Shibayama, S. Nomura)

(6) ポリマーアロイ入門シリーズ　混合状態の解析
　 日本接着協会誌、vol.24, 1988, pp.62-68.
（柴山充弘）

(7) 高強力ＰＶＡの開発動向
　 機能材料、vol.8, 1988, ３月号、pp.16-24.
　（柴山充弘）

(8) Studies on Structure and Properties of High-transparent Polypropylene Film.
Repts. Progr. Polym. Phys. Jpn., vol.31, 1988, pp.179-182.
(D. Takahashi, K. Katoh, M. Shibayama, S. Nomura)

(9) Rheological Studies on Sol-Gel Transition of Poly(vinyl alcohol)-Borate Gel.
Repts. Progr. Polym. Phys. Jpn., vol.32, 1989, pp.87-90.
(H. Kurokawa, M. Shibayama, T. Ishimaru, S. Okamoto, S. Nomura)

(10) Changes in Micro-Structure of Segmented Poly(urethaneurea) in water due to
Mechanical Fatigue.
Repts. Progr. Polym. Phys. Jpn., vol.33, 1990, 319-322.
(S. Kawano, M. Shibayama, S. Nomura)

(11) 小角中性子散乱によるゲルの構造解析
　　表面、vol.29, 1991.5 374-386.
（柴山充弘）

(12) 環境感応型ゲルの体積相転移
　　高分子加工, vol.42, 1993.4, 192-205.
（柴山充弘）

(13) 高分子ゲルの形成と物性
　 ゴム協会誌, vol.66, 1993.4 222-236.
（柴山充弘）

(14) Microscopic View of the Volume Phase Transition on Weakly Charged Temperature
Sensitive Polymer Gels.
Proceeding of the Fifth International Symposium on Advanced Nuclear
Energy Research, vol. 2, 578-585, Mar. 10 -12, Mito, Japan, 1993.
(M. Shibayama, T. Tanaka, C. C. Han)

(15) 高分子ゲル内の不均一構造
　　 表面、vol.31, 1994.2, 117-124.
（柴山充弘）

(16) 荷電高分子ゲルの体積相転移と相分離
　　物性研だより、vol. 36, 1996.2, 38-41.
　 （柴山充弘）

(17) イオン性高分子ゲル
　　繊維学会誌、vol. 52, 1996.10, 409-413.
　（柴山充弘）

(18) Anomalous Cross-Link Density Dependence of Scattering from Charged Gels.
(M. Shibayama, F. Ikkai)
in "Statistical Physics. Experiments, Theories and Computer Similations"
M. Tokuyama, I. Oppenheim, Eds., World Sci.New Jersey, 1998. pp.51.

(19) Spatial Inhomogeneity and Dynamic Fluctuations of Polymer Gels.
Feature Article, Macromol. Chem. Phys. vol. 199, 1-30 (1998).
(M. Shibayama)

(20) Dynamics of Silica Gels in Gelation Process
AIP Conference Series, pp. 85-92 (1999).
(M. Shibayama, Tomohisa Norisuye)

(21) 高分子ゲルの構造解析
　　機能材料、シーエムーシー出版、vol. 19, 1999.1, 7 - 15 .

(22) ゲルのフラクタル解析
　　 高分子、vol. 48, 1999.2, 78-81.

(23)荷電性物理架橋ゲルのゲル化と濃度揺らぎ
表面、vol. 37, 1999.1, 20-28.

(24) 高分子ゲルの空間不均一性
　　高分子加工, vol. 48, 1999.4 155-161.
(F. Ikkai and M. Shibayama)

(25) Small-angle Neutron Scattering on Polymer Gels.
Proceedings of The 1998 Workshop on the Utilization of Research Reactors,
Yogyakarta/Serpong, Indonesia, Feb. 8 - 14, 1999.
Science and Technology Agency of Japan/National Atomic Energy Agency of
Indonesia. pp.131- 142 (1999).
(M. Shibayama)

(26) Small-angle Neutron Scattering on Polymers.
Proceedings of The 1998 Workshop on the Utilization of Research Reactors,
Yogyakarta/Serpong, Indonesia, Feb. 8 - 14, 1999.
Science and Technology Agency of Japan/National Atomic Energy Agency of
Indonesia. pp.411- 472 (1999).
(M. Shibayama)

(26) Spatial Inhomogeneities in Weakly Charged Temperature Sensitive Polymer Gels
in Deformed State
Proceedings of Yamada Conference L, Polyelectrolytes, I. Noda and E. Kokufuta,
Eds. pp. 315- 318 (1999).
(M. Shibayama)

(28) 時分割動的光散乱によるゲル化反応解析
ネットワークポリマー
（柴山充弘）, vol. 20, 1999.3 59-67.

(29) Real-time Observation of Gelation and Vitrification
M. Shibayama, S. Ozeki, and T. Norisuye
Tohwa International Conference on Slow Dynamics, 1999, Fukuoka
Statistical Physics, AIP Conference Proceedings, M. Tokuyama, H. E. Stanley,
Eds., 519, 158-163 (2000).

(30) Gel Formation Analyses by Dynamic Light Scattering
M. Shibayama and T. Norisuye
Bull. Chem., Chem. Soc. Jpn., in press. (2002 April issue).

(31) 分光学的手法による架橋構造解析
ゴム協会誌
(柴山充弘)、vol. 75, 2002.2 62-67.